Magnetic materials for solid-state batteries
Recent progress of magnetic field application in lithium-based
Recently, numerous studies have reported that the use of a magnetic field as a non-contact energy transfer method can effectively improve the electrochemical performance
Solid-State Nuclear Magnetic Resonance Studies of Lithium and
In this review, we first introduce the basics of NMR in studying metal anodes and then select specific examples to illustrate how various NMR methods, including
Recent progress of magnetic field application in lithium-based batteries
It also offers a new strategy for the preparation of other magnetic materials with adjustable magnetic properties. Li et al. [127] prepared a solid polymer electrolyte with high ion conductivity for all-solid-state lithium batteries by mixing PEO with magnetically oriented and functionalized sepiolite (KFSEP) nanowires. Oriented nanowires with high stability have the
Nuclear magnetic resonance for interfaces in rechargeable batteries
Nuclear Magnetic Resonance (NMR) is a powerful technique to probe the local environment of spin-bearing atoms. Recent reviews describe the considerable amount of work related to NMR studies on battery or battery-like devices [1, 2].Following the tradition of this journal, we focus on the reports that were published in the last three years and that shed new
Improving performances of oxide solid electrolytes by a magnetic
All-solid-state lithium-metal batteries have been regarded as the next-generation energy storage due to the potential high safety and high energy density. However, for oxide solid electrolytes (SEs), the relatively low ionic conductivities and the growth of lithium dendrite leading to safety issues limit their commercialization. Here
Advancements and Challenges in Solid-State Battery
Our focus will primarily be on the critical developments in solid electrolytes and anode materials for solid-state batteries (SSBs), with a special emphasis on lithium-metal anodes and their interfaces, elucidating the
Improving performances of oxide solid electrolytes by
All-solid-state lithium-metal batteries have been regarded as the next-generation energy storage due to the potential high safety and high energy density. However, for oxide solid electrolytes (SEs), the relatively low
Advances in solid-state batteries: Materials, interfaces
The primary focus of this article centers on exploring the fundamental principles regarding how electrochemical interface reactions are locally coupled with mechanical and transport properties impacting battery performance, giving opportunities to design electrolyte and interface coating materials for advanced solid-state batteries.
Advances in solid-state batteries: Materials, interfaces
The primary focus of this article centers on exploring the fundamental principles regarding how electrochemical interface reactions are locally coupled with mechanical and transport properties impacting battery performance, giving opportunities to design electrolyte
Recent progress of magnetic field application in lithium-based batteries
Recently, numerous studies have reported that the use of a magnetic field as a non-contact energy transfer method can effectively improve the electrochemical performance of lithium-based batteries relying on the effects of magnetic force, magnetization, magnetohydrodynamic and spin effects.
Recent Advances in Solid-State Nuclear Magnetic Resonance
Establishing structure–property correlations is of paramount importance to materials research. The ability to selectively detect observable magnetization from transitions between quantized spin states of nuclei makes nuclear magnetic resonance (NMR) spectroscopy a powerful probe to characterize solids at the atomic level. In this article, we review recent advances in NMR
Electrolyte and Interface Engineering for Solid-State Sodium Batteries
This review introduces the development and recent progress of different types of solid-state electrolyte for sodium batteries, including β-alumina, NASICON, sulfide-based electrolyte, complex hydrides, and organic electrolyte. In particular, the transport mechanism, ionic conductivity, ionic transference number, chemical/electrochemical stability, and mechanical
Magnetic field-assisted vertically aligned NiFe2O4 nanosheets in
In recent years, all solid-state lithium metal batteries (ASSLMBs) with high energy density and high safety have attracted widespread attention due to their extraordinary potential for academic and industrial communities [1], [2] these ASSLMBs, solid-state electrolytes (SSEs) with high ionic conductivities, wide electrochemical windows and long-term stability play a key role.
A magnetic-assisted construction of functional gradient interlayer
Herein, we designed a functional gradient interlayer (FGIL) with the help of magnetic force to solve the issue of Li dendrite growth on the electrode surface and inside the
A Roadmap for Solid‐State Batteries
Solid-state batteries are considered as a reasonable further development of lithium-ion batteries with liquid electrolytes. While expectations are high, there are still open questions concerning the choice of materials, and the resulting concepts for components and full cells.
Molecular magneto-ionic proton sensor in solid-state proton
Here, we report the proton-based magneto-ionics in molecule-based magnet which serves as both solid-state proton battery electrode and radiofrequency sensing medium.
Enhancing Long Stability of Solid‐State Batteries Through
Metal sulfides are increasingly favored as cathode materials in all-solid-state batteries (ASSBs) due to their high energy density, stability, affordability, and conductivity. Metal sulfides often exhibit capacities exceeding their theoretical limits, a phenomenon that remains not fully understood.
Advancements and Challenges in Solid-State Battery Technology
Our focus will primarily be on the critical developments in solid electrolytes and anode materials for solid-state batteries (SSBs), with a special emphasis on lithium-metal anodes and their interfaces, elucidating the innovative strides in
Improving performances of oxide solid electrolytes by
Yining Zhang, Shaojie Chen, Yue Zhang, Yi Yu, Wei Liu; Improving performances of oxide solid electrolytes by a magnetic field for all-solid-state lithium-metal batteries. Appl. Phys.
Materials'' Methods: NMR in Battery Research
In this Review, we highlight the application of solid-state nuclear magnetic resonance (NMR) spectroscopy in battery research: a technique that can be extremely powerful in characterizing local structures in battery materials, even in highly disordered systems.
Materials'' Methods: NMR in Battery Research
In this Review, we highlight the application of solid-state nuclear magnetic resonance (NMR) spectroscopy in battery research: a technique that can be extremely powerful in characterizing local structures in battery
A cathode homogenization strategy for enabling long-cycle-life all
All-solid-state lithium batteries typically employ heterogeneous composite cathodes where conductive additives are introduced to improve mixed conduction. These electrochemically inactive
Materials and structure engineering by magnetron sputtering for
To lower the contact resistance, Lee and colleagues fabricated an Li-La-Ta-O thin-film electrolyte between a cathode and bulk solid electrolyte via magnetron sputtering to assemble all-solid-state batteries with promising capacities and cycle stabilities.
Solid-State Nuclear Magnetic Resonance Studies of Lithium and
In this review, we first introduce the basics of NMR in studying metal anodes and then select specific examples to illustrate how various NMR methods, including multinuclear magic angle spinning (MAS) NMR, electrochemical in situ NMR, and NMR dynamics methods, provide unique insights into the chemical composition of SEIs, deposit morphological e...
Enhancing Long Stability of Solid‐State Batteries
Metal sulfides are increasingly favored as cathode materials in all-solid-state batteries (ASSBs) due to their high energy density, stability, affordability, and conductivity. Metal sulfides often exhibit capacities
2020 roadmap on solid-state batteries
Within solid-state batteries (SSBs), numerous interfaces exist between electrode active materials and the solid electrolyte. For the practical application of an SSB, minimal impedances between interfacial layers are required. The buried nature of these interfaces presents certain challenges in order to characterise them with traditional surface
Development of solid polymer electrolytes for solid-state lithium
Notably, Jeong and coworkers reviewed the applications of SPEs in all-solid-state lithium batteries, quasi-solid-state lithium batteries, and lithium metal protective layers [15]. In a recent publication in 2023, Wang et al. [ 16 ] primarily focused on block copolymers and provided a summary of the current research status and optimization strategies of block copolymer
Molecular magneto-ionic proton sensor in solid-state proton battery
Here, we report the proton-based magneto-ionics in molecule-based magnet which serves as both solid-state proton battery electrode and radiofrequency sensing medium. The three-dimensional...
A magnetic-assisted construction of functional gradient interlayer
Herein, we designed a functional gradient interlayer (FGIL) with the help of magnetic force to solve the issue of Li dendrite growth on the electrode surface and inside the electrolyte. In the FGIL, the LiF-rich component gathers at the garnet side and the Fe-rich component gathers at the Li side.
Materials and structure engineering by magnetron sputtering for
To lower the contact resistance, Lee and colleagues fabricated an Li-La-Ta-O thin-film electrolyte between a cathode and bulk solid electrolyte via magnetron sputtering to
6 FAQs about [Magnetic materials for solid-state batteries]
What materials can be used in solid-state batteries?
Researchers have been exploring a variety of new materials, including ceramics, polymers, and composites, for their potential in solid-state batteries. These materials offer advantages like better stability and safety compared to traditional liquid electrolytes. Advances in fabrication methods have also been pivotal.
Can magnetic fields be used in lithium-based batteries?
The challenges and future directions of the application of magnetic fields in lithium-based batteries are provided. Lithium-based batteries including lithium-ion, lithium-sulfur, and lithium-oxygen batteries are currently some of the most competitive electrochemical energy storage technologies owing to their outstanding electrochemical performance.
Are anode materials compatible with solid-state batteries?
The review emphasizes the criticality of considering anode materials’ compatibility with solid-state batteries (SSBs). It underlines the importance of anode stability in solid-state environments to preserve the integrity of the solid electrolyte and avert degradation.
Can solid electrolytes be used in solid-state batteries?
The field of solid electrolytes has seen significant strides due to innovations in materials and fabrication methods. Researchers have been exploring a variety of new materials, including ceramics, polymers, and composites, for their potential in solid-state batteries.
What makes a battery a solid state battery?
2. Solid Electrolytes: The Heart of Solid-State Batteries The gradual shift to solid electrolytes has been influenced by the prior development of conventional lithium (Li) batteries, which have traditionally employed liquid electrolytes.
Does molecule-based magnet serve as a solid-state proton battery electrode?
Despite such promise, the realization of proton magneto-ionics is hampered by the lack of proton-responsive magnets as well as the solid-state sensing method. Here, we report the proton-based magneto-ionics in molecule-based magnet which serves as both solid-state proton battery electrode and radiofrequency sensing medium.
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